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Relation Between n2 and Two-Photon Absorption Pages: 7 Published: Jan 1990
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View License Agreement Source: STP1117-EB Abstract We present evidence from nonlinear refractive index measurements, two-photon absorption measurements, and fourwave mixing measurements on semiconductors showing that the bound electronic nonlinearity can be calculated from two-photon absorption dispersion via a simple Kramers-Kronig analysis. This analysis shows n2 changing from positive to negative as the photon energy approaches the band-gap energy, consistent with observations. Additionally, this simple calculation, which assumes two parabolic bands, gives good agreement with measured values of n2 in wide-gap dielectrics that are 2 to 3 orders of magnitude smaller than in semiconductors. Keywords: nonlinear refraction, two-photon absorption, Kramers-Kronig, four-wave mixing, semiconductors Paper ID: STP26525S Committee/Subcommittee: E13.15 DOI: 10.1520/STP26525S ASTM International is a member of CrossRef. | ||